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Self-aligned Hybrid Nanocavities Using Atomically Thin Materials

ACS PHOTONICS(2024)

RIKEN Cluster Pioneering Res | RIKEN Ctr Adv Photon | Natl Inst Mat Sci

Cited 0|Views17
Abstract
Two-dimensional (2D) materials are increasingly being adopted in hybrid photonics via integration with photonic structures, including cavities. The utility of 2D materials for dielectric environment engineering in hybrid nanophotonic devices remains largely unexplored. We demonstrate self-aligned hybrid nanocavities in which 2D material flakes are used to form cavities locally wherever they are placed along the PhC waveguide postfabrication. We successfully fabricated such hybrid nanocavities with various 2D materials on silicon PhC waveguides, obtaining Q factors as high as 4.0 x 10(5). Remarkably, even monolayer flakes can provide sufficient local refractive index modulation to induce high Q nanocavity formation. We have also observed cavity PL enhancement in a self-aligned MoTe2 cavity device with an enhancement factor of about 15. Our results highlight the prospect of using such 2D material-induced PhC nanocavities to realize a wide range of photonic components for hybrid integrated photonic circuits.
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photonic crystal,hexagonal boron nitride,transition metal dichalcogenide,light-matter interaction
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要点】:本论文展示了一种新方法,通过在硅基光子晶体波导上后处理覆盖合适的二维材料碎片,实现了自对准混合纳米腔的制备,该方法避免了传统预先制造光子晶体纳米腔的复杂性,并且不会降低腔体的品质因子(Q因子)。创新点在于二维材料与光子结构的集成实现了高质量的光 matter 耦合。

方法】:研究采用了一种新颖的方法,通过在硅基光子晶体波导上后处理,部分覆盖了由原子层厚材料制成的碎片来形成混合纳米腔。

实验】:实验中使用了氮化硼(hBN)、二维过渡金属硫化物(WSe₂和MoTe₂)碎片与硅基光子晶体波导结合,成功制备了混合纳米腔设备,获得了高达4.0×10^5的品质因子(Q因子)。即使是一层或几层厚的碎片也足以提供足够的局部折射率调制,从而诱导纳米腔的形成。由于二维材料与纳米腔自对准,研究观察到MoTe₂混合腔设备的腔体发光增强,其腔体浦尔凯尔增强因子约为15。