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Coulomb Interactions and Migrating Dirac Cones Imaged by Local Quantum Oscillations in Twisted Graphene

Nature physics(2025)

Cited 0|Views9
Abstract
Flat-band moiré graphene systems are a quintessential platform for investigating correlated phases of matter. Various interaction-driven ground states have been proposed, but despite extensive experimental effort, there has been little direct evidence that distinguishes between various phases, in particular near the charge neutrality point. Here we probe the fine details of the density of states and the effects of Coulomb interactions in alternating-twist trilayer graphene by imaging the local thermodynamic quantum oscillations with a nanoscale scanning superconducting quantum interference device. We find that the charging self-energy due to occupied electronic states is most important in explaining the high-carrier-density physics. At half-filling of the conduction flat band, we observe ferromagnetic-driven symmetry breaking, suggesting that it is the most robust mechanism in the hierarchy of phase transitions. Near charge neutrality, where exchange energy dominates over charging self-energy, we find a nematic semimetal ground state, which is theoretically favoured over gapped states in the presence of heterostrain. In this semimetallic phase, the flat-band Dirac cones migrate towards the mini-Brillouin zone centre, spontaneously breaking the threefold rotational symmetry. Our low-field local quantum oscillation technique can be used to explore the ground states of many strongly interacting van der Waals systems.
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要点】:本文利用纳米级扫描超导量子干涉器在扭曲三层石墨烯中成像局部热力学量子振荡,揭示了库仑相互作用和迁移的狄拉克锥,发现了近中性点处的电荷密度对称性破缺现象。

方法】:通过纳米级扫描超导量子干涉器在极低磁场下(56 mT)成像局部热力学量子振荡,研究了电子态密度和单粒子能带结构受库仑相互作用的修正。

实验】:实验使用交替扭曲的三层石墨烯作为样品,在低磁场下观测到电荷中性点附近的半填充导带平坦带中Stoner-like对称性破缺,并在接近电荷中性点时发现电荷中性态为nematic半金属材料,其狄拉克锥向迷你布里渊区中心迁移,实验结果揭示了库仑相互作用在电荷密度物理中的关键作用。